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Löwenburg Castle (or Kassel Wilhelmshöhe in German translated as “Lion’s Castle”) is unique among all the castles in Germany in that it was conceived as a romantic medieval castle ruin. The design of Löwenburg Castle was based on a fantasy of Landgrave Wilhelm IX, but experts regard it a very important historical monument, because it was the first neogothic structure in the country.

Schloss Falkenstein - Ludwig II's design for another fairy tale castle to top even Neuschwanstein. Check out his Wiki page:

Schloss Buerresheim castle in Germany. Used in Indiana Jones and The Last Crusade as Castle Brunwald.